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Can you explain your use case so that we can understand what it is you want to do?
For one, I'd like to know if by attribute and values that you mean either AFAttribute and AFValues, or do you mean PIPoint Attributes with their name and value pairs? If you mean AFAttribute, then a name by itself may not be sufficiently unique. You may need its path, relative to the database or perhaps the full path including asset server.
For working with code, a dictionary may be preferred over a DataTable. So it would help to know what you were planning on doing later with this table.